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Wang,  Huihui

Laser-driven electron and spin-state quantum dynamics in transition metal complexes

Rostock : Universität , 2018

https://doi.org/10.18453/rosdok_id00002338

http://purl.uni-rostock.de/rosdok/id00002338

Recent advances in attosecond spectroscopy open the door to the understanding correlated motion of valence and core electrons in molecular systems. In this thesis, the density matrix-based TD-RASCI method is used to study the electron and spin-flip dynamics. The dephasing effect of nuclear vibrations is incorporated implicitly making use of an electronic system/vibrational bath partitioning. We theoretically addressed the ultrafast spin-flip dynamics in a transition metal complex which is triggered by isolated sub-fs soft-X-ray pulses as well as X-ray pulse trains.

Dissertation Open Access


Einrichtung :
Mathematisch-Naturwissenschaftliche Fakultät
Gutachter :
Vendrell,  Oriol
Kühn,  Oliver
Bokarev,  Sergey
Sprache(n) :
Englisch
DDC Klassifikation :
530 Physik
URN :
urn:nbn:de:gbv:28-diss2018-0166-0
Persistente URL:
http://purl.uni-rostock.de/rosdok/id00002338
erstellt am:
2018-11-26
zuletzt geändert am:
2018-11-26
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