mycoreobjectrosdok_disshab_0000001403rosdok_disshab_0000001403rosdokdisshabrosdok_derivate_00000288992023-08-08T10:06:08.102Z2015-08-05T13:42:30.972ZadministratoreditorDpublished1rosdok_derivate_0000028899truetruederivate_types:fulltextVolltextfulltextwf_edit_epub wf_register_epubstate:publishedstate:publishedveröffentlichtpublishedrosdok/id00001582833612840MODS updated during RosDok migration in June 2021DissertationHochschulschrift1075019915MateuszLisaj1986-VerfasserInautLaser control and spectroscopy of molecular vibrations and reaction dynamicsen141056487Prof. Dr.OliverKühnUniversität Rostock, Institut für PhysikAkademischeR BetreuerIndgs110000625PD Dr. habil.VolkhardMayHumboldt-Universität zu Berlin, Institut für PhysikAkademischeR BetreuerIndgs2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg10.18453/rosdok_id00001582http://purl.uni-rostock.de/rosdok/id00001582urn:nbn:de:gbv:28-diss2015-0132-4530 PhysikMathematisch-Naturwissenschaftliche Fakultätfrei zugänglich (Open Access)Lizenz Metadaten: CC0Nutzungsrechte erteiltalle Rechte vorbehaltenUniversität RostockRostock2015monographic20152015Universitätsbibliothek RostockRostock20152015The main subjects of this work are the ultrafast laser driven quantum dynamics of collective CO vibrations in a metal-dicarbonyl complex. The fundamental insights into the interactions responsible for bond dissociation are obtained by using shaped laser pulses to steer molecular quantum dynamics. Specifically, CpCo(CO)2 is studied on the basis of a four-dimensional reactive potential energy surface (PES). It is shown that two perpendicularly polarized IR laser pulses can be used to trigger an alternating localization of the vibration within one CO bond.femtosecond IR pulsesmetal-carbonyl complexesalcoholysis reactionsbond breakingtransient localizationwave packet dynamicsUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00001582doctype:epubdoctype:epubDokumenttypDocument typedoctype:epub.dissertationdoctype:epub.dissertationDissertationdoctoral thesisdiniPublType:doctoralThesis diniPublType2022:PhDThesis XMetaDissPlusThesisLevel:thesis.doctoralinfo:eu-repo/semantics/doctoralThesisdocumentnatureOfContent:ppn_105825778natureOfContent:ppn_105825778HochschulschriftdiniPublType2022:DoctoralThesisdiniPublType2022:DoctoralThesisDissertation oder HabilitationDoctoral thesisDRIVERdiniPublType2022:PhDThesisdiniPublType2022:PhDThesisDissertationPhD thesisKDSF (Pu34)XMetaDissPlusThesisLevel:thesis.doctoralXMetaDissPlusThesisLevel:thesis.doctoralDoktorarbeitdoctoral thesisrfc5646:enrfc5646:enEnglischEnglishengengSDNB:530SDNB:530530 Physik530 Physicsinstitution:unirostockinstitution:unirostockUniversität RostockUniversity of RostockUniversität RostockUniversität RostockUni.Rostockhttp://d-nb.info/gnd/38329-6institution:unirostock.mnfinstitution:unirostock.mnfMathematisch-Naturwissenschaftliche FakultätFaculty of Mathematics and Natural SciencesUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätMathematisch-Natur-<br />wissenschaftliche FakultätUni.Rostock.Fakultaet.MNFhttp://d-nb.info/gnd/2147083-2accesscondition:openaccessaccesscondition:openaccessfrei zugänglich (Open Access)open accesshttp://purl.org/coar/access_right/c_abf2OAfreeinfo:eu-repo/semantics/openAccess[DE-28]Open Access$gControlled Vocabulary for Access Rights$uhttp://purl.org/coar/access_right/c_abf2licenseinfo:metadatalicenseinfo:metadataLizenzen für Metadatenlicenseinfo:metadata.cc0licenseinfo:metadata.cc0Lizenz Metadaten: CC0license metadata: CC0/creativecommons/p/zero/1.0/88x31.pnghttps://creativecommons.org/publicdomain/zero/1.0/licenseinfo:depositlicenseinfo:depositVeröffentlichungsgenehmigungpermission to storelicenseinfo:deposit.rightsgrantedlicenseinfo:deposit.rightsgrantedNutzungsrechte erteiltrights grantedlicenseinfo:worklicenseinfo:workWerkworklicenseinfo:work.rightsreservedlicenseinfo:work.rightsreservedalle Rechte vorbehaltenall rights reserved/creativecommons/r/reserved/0.9/88x31.png[DE-28]Urheberrechtsschutz 1.0$gRights Statements$uhttp://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/Laser control and spectroscopy of molecular vibrations and reaction dynamicsLaser control and spectroscopy of molecular vibrations and reaction dynamicsgnd:1075019915gnd:141056487gnd:110000625gnd:2147083-2gnd:1075019915gnd:141056487gnd:110000625gnd:2147083-2rosdok_disshab_0000001403-d61678e39gnd:1075019915Mateusz LisajMateusz Lisajrosdok_disshab_0000001403-d61678e60gnd:141056487Prof. Dr. Oliver KühnProf. Dr. Oliver Kühnrosdok_disshab_0000001403-d61678e75gnd:110000625PD Dr. habil. Volkhard MayPD Dr. habil. Volkhard Mayrosdok_disshab_0000001403-d61678e90gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätMateusz LisajProf. Dr. Oliver KühnPD Dr. habil. Volkhard MayUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätMateusz LisajProf. Dr. Oliver KühnPD Dr. habil. Volkhard MayUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätMateusz LisajRostockUniversität Rostockepub.dissertation10.18453/rosdok_id00001582http://purl.uni-rostock.de/rosdok/id00001582urn:nbn:de:gbv:28-diss2015-0132-4femtosecond IR pulsesmetal-carbonyl complexesalcoholysis reactionsbond breakingtransient localizationwave packet dynamicsThe main subjects of this work are the ultrafast laser driven quantum dynamics of collective CO vibrations in a metal-dicarbonyl complex. The fundamental insights into the interactions responsible for bond dissociation are obtained by using shaped laser pulses to steer molecular quantum dynamics. Specifically, CpCo(CO)2 is studied on the basis of a four-dimensional reactive potential energy surface (PES). It is shown that two perpendicularly polarized IR laser pulses can be used to trigger an alternating localization of the vibration within one CO bond.20152015epub.dissertation1 Dissertation_Lisaj_2015.pdf 18622042 05eab9eb202dbaa53f43a678a9b3e9c4 rosdok/id00001582833612840MODS updated during RosDok migration in June 2021DissertationHochschulschrift1075019915MateuszLisaj1986-VerfasserInautLaser control and spectroscopy of molecular vibrations and reaction dynamicsen141056487Prof. Dr.OliverKühnUniversität Rostock, Institut für PhysikAkademischeR BetreuerIndgs110000625PD Dr. habil.VolkhardMayHumboldt-Universität zu Berlin, Institut für PhysikAkademischeR BetreuerIndgs2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg10.18453/rosdok_id00001582http://purl.uni-rostock.de/rosdok/id00001582urn:nbn:de:gbv:28-diss2015-0132-4530 PhysikMathematisch-Naturwissenschaftliche Fakultätfrei zugänglich (Open Access)Lizenz Metadaten: CC0Nutzungsrechte erteiltalle Rechte vorbehaltenUniversität RostockRostock2015monographic20152015Universitätsbibliothek RostockRostock20152015The main subjects of this work are the ultrafast laser driven quantum dynamics of collective CO vibrations in a metal-dicarbonyl complex. The fundamental insights into the interactions responsible for bond dissociation are obtained by using shaped laser pulses to steer molecular quantum dynamics. Specifically, CpCo(CO)2 is studied on the basis of a four-dimensional reactive potential energy surface (PES). It is shown that two perpendicularly polarized IR laser pulses can be used to trigger an alternating localization of the vibration within one CO bond.femtosecond IR pulsesmetal-carbonyl complexesalcoholysis reactionsbond breakingtransient localizationwave packet dynamicsUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00001582 2015-08-05T13:42:30.972Z 2023-08-08T10:06:08.102Z 2023-08-18T10:06:08.107Z editorD {"identifier":"rosdok/id00001582","type":"local_id","additional":"","service":"MCRLocalID","created":"2018-06-30T13:17:39.716Z"} {"identifier":"http://purl.uni-rostock.de/rosdok/id00001582","type":"purl","additional":"","service":"RosDokPURL","created":"2018-06-30T13:17:39.904Z","registered":"2018-06-30T13:17:39.904Z"} {"identifier":"10.18453/rosdok_id00001582","type":"doi","additional":"","service":"RosDokDOI","created":"2018-06-30T13:17:42.697Z","registered":"2018-06-30T13:17:42.697Z"} {"identifier":"urn:nbn:de:gbv:28-diss2015-0132-4","type":"dnbUrn","additional":"","service":"RosDokURN","created":"2018-06-30T13:17:39.722Z","registered":"2015-08-22T02:23:14.667Z"} administratorfulltextfile/rosdok_disshab_0000001403/rosdok_derivate_0000028899/Dissertation_Lisaj_2015.pdfLaser control and spectroscopy of molecular vibrations and reaction dynamicsLaser control and spectroscopy of molecular vibrations and reaction dynamicsgnd:1075019915gnd:141056487gnd:110000625gnd:2147083-2gnd:1075019915gnd:141056487gnd:110000625gnd:2147083-2rosdok_disshab_0000001403-d61678e39gnd:1075019915Mateusz LisajMateusz Lisajrosdok_disshab_0000001403-d61678e60gnd:141056487Prof. Dr. Oliver KühnProf. Dr. Oliver Kühnrosdok_disshab_0000001403-d61678e75gnd:110000625PD Dr. habil. Volkhard MayPD Dr. habil. Volkhard Mayrosdok_disshab_0000001403-d61678e90gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätMateusz LisajProf. Dr. Oliver KühnPD Dr. habil. Volkhard MayUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätMateusz LisajProf. Dr. Oliver KühnPD Dr. habil. Volkhard MayUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätMateusz LisajRostockUniversität Rostockepub.dissertation10.18453/rosdok_id00001582http://purl.uni-rostock.de/rosdok/id00001582urn:nbn:de:gbv:28-diss2015-0132-4femtosecond IR pulsesmetal-carbonyl complexesalcoholysis reactionsbond breakingtransient localizationwave packet dynamicsThe main subjects of this work are the ultrafast laser driven quantum dynamics of collective CO vibrations in a metal-dicarbonyl complex. The fundamental insights into the interactions responsible for bond dissociation are obtained by using shaped laser pulses to steer molecular quantum dynamics. Specifically, CpCo(CO)2 is studied on the basis of a four-dimensional reactive potential energy surface (PES). It is shown that two perpendicularly polarized IR laser pulses can be used to trigger an alternating localization of the vibration within one CO bond.20152015[xslt]Saxonrosdok/id00001582https://purl.uni-rostock.de/rosdok/id0000158283361284010.18453/rosdok_id00001582urn:nbn:de:gbv:28-diss2015-0132-4Mateusz LisajLisaj MateuszLaser control and spectroscopy of molecular vibrations and reaction dynamicsDissertationdoctoral thesisUniversität Rostock, 2015The main subjects of this work are the ultrafast laser driven quantum dynamics of collective CO vibrations in a metal-dicarbonyl complex. The fundamental insights into the interactions responsible for bond dissociation are obtained by using shaped laser pulses to steer molecular quantum dynamics.…Mateusz LisajLaser control and spectroscopy of molecular vibrations and reaction dynamicsUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id000015821075019915MateuszLisaj1986-VerfasserInaut141056487Prof. Dr.OliverKühnUniversität Rostock, Institut für PhysikAkademischeR BetreuerIndgs110000625PD Dr. habil.VolkhardMayHumboldt-Universität zu Berlin, Institut für PhysikAkademischeR BetreuerIndgs2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg[doi]10.18453/rosdok_id00001582[purl]http://purl.uni-rostock.de/rosdok/id00001582[urn]urn:nbn:de:gbv:28-diss2015-0132-4open_access20152015epoch:21th_centuryrfc5646:endoctype:epub.dissertationaccesscondition:openaccessSDNB:530institution:unirostock.mnfstate:published