mycoreobjectrosdok_disshab_0000001425rosdok_disshab_0000001425rosdokdisshabrosdok_derivate_00000290892023-08-08T10:06:14.609Z2015-08-24T10:34:54.176ZadministratoreditorDpublished1rosdok_derivate_0000029089truetruederivate_types:fulltextVolltextfulltextwf_edit_epub wf_register_epubstate:publishedstate:publishedveröffentlichtpublishedrosdok/id00001604833962744MODS updated during RosDok migration in June 2021DissertationHochschulschrift107574184XJacqueline BettinaPriebe1985-VerfasserInautStructure-reactivity relationships in plasmonic metal-semiconductor nanocomposites for photocatalytic hydrogen generation assessed by in situ spectroscopyen14344526XProf. Dr.AngelikaBrücknerLeibniz-Institut für Katalyse e.V. an der Universität Rostock, Bereich für katalytische in situ-StudienAkademischeR BetreuerIndgsProf. Dr.MichaelWarkCarl von Ossietzky Universität Oldenburg, Institut für Chemie - Technische ChemieAkademischeR BetreuerIndgsProf. Dr.MatthiasBauerUniversität Paderborn, Institut für Chemie - Anorganische und Analytische ChemieAkademischeR BetreuerIndgs2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg10.18453/rosdok_id00001604http://purl.uni-rostock.de/rosdok/id00001604urn:nbn:de:gbv:28-diss2015-0154-7540 ChemieMathematisch-Naturwissenschaftliche Fakultätfrei zugänglich (Open Access)Lizenz Metadaten: CC0Nutzungsrechte erteiltalle Rechte vorbehaltenUniversität RostockRostock2015monographic20152015Universitätsbibliothek RostockRostock20152015This work addresses photocatalytic generation of hydrogen (H2) from water and methanol over semiconductor-supported metal catalysts, such as Au, Ag and Cu, allowing proton reduction under visible light. Structure-reactivity relationships were assessed by applying suitable in situ spectroscopic techniques and by varying the composition of the semiconductor as well as of the metal component. It was shown that the ability of charge-carrier formation and transfer was strongly affected by the support properties, such as surface area, defects or surface-trapping sites.In-situ-SpektroskopiePhotokatalyseWasserstofferzeugungUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00001604doctype:epubdoctype:epubDokumenttypDocument typedoctype:epub.dissertationdoctype:epub.dissertationDissertationdoctoral thesisdiniPublType:doctoralThesis diniPublType2022:PhDThesis XMetaDissPlusThesisLevel:thesis.doctoralinfo:eu-repo/semantics/doctoralThesisdocumentnatureOfContent:ppn_105825778natureOfContent:ppn_105825778HochschulschriftdiniPublType2022:DoctoralThesisdiniPublType2022:DoctoralThesisDissertation oder HabilitationDoctoral thesisDRIVERdiniPublType2022:PhDThesisdiniPublType2022:PhDThesisDissertationPhD thesisKDSF (Pu34)XMetaDissPlusThesisLevel:thesis.doctoralXMetaDissPlusThesisLevel:thesis.doctoralDoktorarbeitdoctoral thesisrfc5646:enrfc5646:enEnglischEnglishengengSDNB:540SDNB:540540 Chemie540 Chemistry & allied sciencesinstitution:unirostockinstitution:unirostockUniversität RostockUniversity of RostockUniversität RostockUniversität RostockUni.Rostockhttp://d-nb.info/gnd/38329-6institution:unirostock.mnfinstitution:unirostock.mnfMathematisch-Naturwissenschaftliche FakultätFaculty of Mathematics and Natural SciencesUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätMathematisch-Natur-<br />wissenschaftliche FakultätUni.Rostock.Fakultaet.MNFhttp://d-nb.info/gnd/2147083-2accesscondition:openaccessaccesscondition:openaccessfrei zugänglich (Open Access)open accesshttp://purl.org/coar/access_right/c_abf2OAfreeinfo:eu-repo/semantics/openAccess[DE-28]Open Access$gControlled Vocabulary for Access Rights$uhttp://purl.org/coar/access_right/c_abf2licenseinfo:metadatalicenseinfo:metadataLizenzen für Metadatenlicenseinfo:metadata.cc0licenseinfo:metadata.cc0Lizenz Metadaten: CC0license metadata: CC0/creativecommons/p/zero/1.0/88x31.pnghttps://creativecommons.org/publicdomain/zero/1.0/licenseinfo:depositlicenseinfo:depositVeröffentlichungsgenehmigungpermission to storelicenseinfo:deposit.rightsgrantedlicenseinfo:deposit.rightsgrantedNutzungsrechte erteiltrights grantedlicenseinfo:worklicenseinfo:workWerkworklicenseinfo:work.rightsreservedlicenseinfo:work.rightsreservedalle Rechte vorbehaltenall rights reserved/creativecommons/r/reserved/0.9/88x31.png[DE-28]Urheberrechtsschutz 1.0$gRights Statements$uhttp://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/Structure-reactivity relationships in plasmonic metal-semiconductor nanocomposites for photocatalytic hydrogen generation assessed by in situ spectroscopyStructure-reactivity relationships in plasmonic metal-semiconductor nanocomposites for photocatalytic hydrogen generation assessed by in situ spectroscopygnd:107574184Xgnd:14344526Xgnd:2147083-2gnd:107574184Xgnd:14344526Xgnd:2147083-2rosdok_disshab_0000001425-d2784126e39gnd:107574184XJacqueline Bettina PriebeJacqueline Bettina Prieberosdok_disshab_0000001425-d2784126e60gnd:14344526XProf. Dr. Angelika BrücknerProf. Dr. Angelika Brücknerrosdok_disshab_0000001425-d2784126e75Prof. Dr. Michael WarkProf. Dr. Michael Warkrosdok_disshab_0000001425-d2784126e88Prof. Dr. Matthias BauerProf. Dr. Matthias Bauerrosdok_disshab_0000001425-d2784126e102gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätJacqueline Bettina PriebeProf. Dr. Angelika BrücknerProf. Dr. Michael WarkProf. Dr. Matthias BauerUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätJacqueline Bettina PriebeProf. Dr. Angelika BrücknerProf. Dr. Michael WarkProf. Dr. Matthias BauerUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätJacqueline Bettina PriebeRostockUniversität Rostockepub.dissertation10.18453/rosdok_id00001604http://purl.uni-rostock.de/rosdok/id00001604urn:nbn:de:gbv:28-diss2015-0154-7In-situ-SpektroskopiePhotokatalyseWasserstofferzeugungThis work addresses photocatalytic generation of hydrogen (H2) from water and methanol over semiconductor-supported metal catalysts, such as Au, Ag and Cu, allowing proton reduction under visible light. Structure-reactivity relationships were assessed by applying suitable in situ spectroscopic techniques and by varying the composition of the semiconductor as well as of the metal component. It was shown that the ability of charge-carrier formation and transfer was strongly affected by the support properties, such as surface area, defects or surface-trapping sites.20152015epub.dissertation1 Dissertation_Priebe_2015.pdf 22180306 af0b05a27458dad04935ebbb55a3f704 rosdok/id00001604833962744MODS updated during RosDok migration in June 2021DissertationHochschulschrift107574184XJacqueline BettinaPriebe1985-VerfasserInautStructure-reactivity relationships in plasmonic metal-semiconductor nanocomposites for photocatalytic hydrogen generation assessed by in situ spectroscopyen14344526XProf. Dr.AngelikaBrücknerLeibniz-Institut für Katalyse e.V. an der Universität Rostock, Bereich für katalytische in situ-StudienAkademischeR BetreuerIndgsProf. Dr.MichaelWarkCarl von Ossietzky Universität Oldenburg, Institut für Chemie - Technische ChemieAkademischeR BetreuerIndgsProf. Dr.MatthiasBauerUniversität Paderborn, Institut für Chemie - Anorganische und Analytische ChemieAkademischeR BetreuerIndgs2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg10.18453/rosdok_id00001604http://purl.uni-rostock.de/rosdok/id00001604urn:nbn:de:gbv:28-diss2015-0154-7540 ChemieMathematisch-Naturwissenschaftliche Fakultätfrei zugänglich (Open Access)Lizenz Metadaten: CC0Nutzungsrechte erteiltalle Rechte vorbehaltenUniversität RostockRostock2015monographic20152015Universitätsbibliothek RostockRostock20152015This work addresses photocatalytic generation of hydrogen (H2) from water and methanol over semiconductor-supported metal catalysts, such as Au, Ag and Cu, allowing proton reduction under visible light. Structure-reactivity relationships were assessed by applying suitable in situ spectroscopic techniques and by varying the composition of the semiconductor as well as of the metal component. It was shown that the ability of charge-carrier formation and transfer was strongly affected by the support properties, such as surface area, defects or surface-trapping sites.In-situ-SpektroskopiePhotokatalyseWasserstofferzeugungUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00001604 2015-08-24T10:34:54.176Z 2023-08-08T10:06:14.609Z 2023-08-18T10:06:14.613Z editorD {"identifier":"rosdok/id00001604","type":"local_id","additional":"","service":"MCRLocalID","created":"2018-06-30T13:18:27.190Z"} {"identifier":"http://purl.uni-rostock.de/rosdok/id00001604","type":"purl","additional":"","service":"RosDokPURL","created":"2018-06-30T13:18:27.423Z","registered":"2018-06-30T13:18:27.423Z"} {"identifier":"10.18453/rosdok_id00001604","type":"doi","additional":"","service":"RosDokDOI","created":"2018-06-30T13:18:28.700Z","registered":"2018-06-30T13:18:28.700Z"} {"identifier":"urn:nbn:de:gbv:28-diss2015-0154-7","type":"dnbUrn","additional":"","service":"RosDokURN","created":"2018-06-30T13:18:27.223Z","registered":"2015-08-27T02:23:09.463Z"} administratorfulltextfile/rosdok_disshab_0000001425/rosdok_derivate_0000029089/Dissertation_Priebe_2015.pdfStructure-reactivity relationships in plasmonic metal-semiconductor nanocomposites for photocatalytic hydrogen generation assessed by in situ spectroscopyStructure-reactivity relationships in plasmonic metal-semiconductor nanocomposites for photocatalytic hydrogen generation assessed by in situ spectroscopygnd:107574184Xgnd:14344526Xgnd:2147083-2gnd:107574184Xgnd:14344526Xgnd:2147083-2rosdok_disshab_0000001425-d2784126e39gnd:107574184XJacqueline Bettina PriebeJacqueline Bettina Prieberosdok_disshab_0000001425-d2784126e60gnd:14344526XProf. Dr. Angelika BrücknerProf. Dr. Angelika Brücknerrosdok_disshab_0000001425-d2784126e75Prof. Dr. Michael WarkProf. Dr. Michael Warkrosdok_disshab_0000001425-d2784126e88Prof. Dr. Matthias BauerProf. Dr. Matthias Bauerrosdok_disshab_0000001425-d2784126e102gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätJacqueline Bettina PriebeProf. Dr. Angelika BrücknerProf. Dr. Michael WarkProf. Dr. Matthias BauerUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätJacqueline Bettina PriebeProf. Dr. Angelika BrücknerProf. Dr. Michael WarkProf. Dr. Matthias BauerUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätJacqueline Bettina PriebeRostockUniversität Rostockepub.dissertation10.18453/rosdok_id00001604http://purl.uni-rostock.de/rosdok/id00001604urn:nbn:de:gbv:28-diss2015-0154-7In-situ-SpektroskopiePhotokatalyseWasserstofferzeugungThis work addresses photocatalytic generation of hydrogen (H2) from water and methanol over semiconductor-supported metal catalysts, such as Au, Ag and Cu, allowing proton reduction under visible light. Structure-reactivity relationships were assessed by applying suitable in situ spectroscopic techniques and by varying the composition of the semiconductor as well as of the metal component. It was shown that the ability of charge-carrier formation and transfer was strongly affected by the support properties, such as surface area, defects or surface-trapping sites.20152015[xslt]Saxonrosdok/id00001604https://purl.uni-rostock.de/rosdok/id0000160483396274410.18453/rosdok_id00001604urn:nbn:de:gbv:28-diss2015-0154-7Jacqueline Bettina PriebePriebe Jacqueline BettinaStructure-reactivity relationships in plasmonic metal-semiconductor nanocomposites for photocatalytic hydrogen generation assessed by in situ spectroscopyDissertationdoctoral thesisUniversität Rostock, 2015This work addresses photocatalytic generation of hydrogen (H2) from water and methanol over semiconductor-supported metal catalysts, such as Au, Ag and Cu, allowing proton reduction under visible light. Structure-reactivity relationships were assessed by applying suitable in situ spectroscopic…Jacqueline Bettina PriebeStructure-reactivity relationships in plasmonic metal-semiconductor nanocomposites for photocatalytic hydrogen generation assessed by in situ spectroscopyUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00001604107574184XJacqueline BettinaPriebe1985-VerfasserInaut14344526XProf. Dr.AngelikaBrücknerLeibniz-Institut für Katalyse e.V. an der Universität Rostock, Bereich für katalytische in situ-StudienAkademischeR BetreuerIndgsProf. Dr.MichaelWarkCarl von Ossietzky Universität Oldenburg, Institut für Chemie - Technische ChemieAkademischeR BetreuerIndgsProf. Dr.MatthiasBauerUniversität Paderborn, Institut für Chemie - Anorganische und Analytische ChemieAkademischeR BetreuerIndgs2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg[doi]10.18453/rosdok_id00001604[purl]http://purl.uni-rostock.de/rosdok/id00001604[urn]urn:nbn:de:gbv:28-diss2015-0154-7open_access20152015epoch:21th_centuryrfc5646:endoctype:epub.dissertationaccesscondition:openaccessSDNB:540institution:unirostock.mnfstate:published