mycoreobjectrosdok_disshab_0000002221rosdok_disshab_0000002221rosdokdisshabrosdok_derivate_00000819542023-08-08T10:10:52.807Z2020-01-10T10:23:12.838ZadministratoreditorDpublished1rosdok_derivate_0000081954truetruederivate_types:fulltextVolltextfulltextwf_edit_epub wf_register_epubstate:publishedstate:publishedveröffentlichtpublishedrosdok/id000025941687013330Oau2020-01-102023-08-05T19:13:53ZrdaConverted from PICA to MODS using Pica2Mods XSLT Transformer 2.7 [SCM: "0c0e7a3c226a4a0cbcbec39b493c3c5257339ab8" "v2.7" "2023-08-04T00:00:00+0200"] with mode 'DEFAULT'.DissertationHochschulschriftCopper catalyzed sun fuel generation by CO2 and H2O reductionHeterogeneous copper-based catalysts have been investigated for the photocatalytic H2O and CO2 reduction. Ex situ and in situ synthesized catalysts supported on inert silica have been developed for the photocatalytic proton reduction. The best supported photocatalyst achieved a significantly higher activity compared to the initial homogeneous precursor. In a second project highly porous photocatalysts have been synthesized, applied in aqueous CO2 reduction and characterized by in situ XAS, EPR and UV-vis measurements. An improved catalytic performance was observed by the addition of oxygen.StefanieKreft1985 -VerfasserInaut1202554695MatthiasBeller1962 -AkademischeR BetreuerIndgs1120819080000-0001-5709-0965RalfLudwig1961 -AkademischeR BetreuerIndgs13643752438329-6Universität Rostock1419 -Grad-verleihende Institutiondgg2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttp://purl.uni-rostock.de/rosdok/id00002594urn:nbn:de:gbv:28-rosdok_id00002594-810.18453/rosdok_id00002594540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en2019Universität RostockRostockmonographic201920192020Universitätsbibliothek RostockRostock2020Universitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00002594Matthias Beller (Universität Rostock, Leibniz-Institut für Katalyse e.V.) ; Ralf Ludwig (Universität Rostock, Institut für Chemie)Enthält Zeitschriftenartikelvorgelegt von Stefanie KreftFotokatalyseReduktionEnergieerzeugungKatalysatordoctype:epubdoctype:epubDokumenttypDocument typedoctype:epub.dissertationdoctype:epub.dissertationDissertationdoctoral thesisdiniPublType:doctoralThesis diniPublType2022:PhDThesis XMetaDissPlusThesisLevel:thesis.doctoralinfo:eu-repo/semantics/doctoralThesisdocumentnatureOfContent:ppn_105825778natureOfContent:ppn_105825778HochschulschriftdiniPublType2022:DoctoralThesisdiniPublType2022:DoctoralThesisDissertation oder HabilitationDoctoral thesisDRIVERdiniPublType2022:PhDThesisdiniPublType2022:PhDThesisDissertationPhD thesisKDSF (Pu34)XMetaDissPlusThesisLevel:thesis.doctoralXMetaDissPlusThesisLevel:thesis.doctoralDoktorarbeitdoctoral thesisSDNB:540SDNB:540540 Chemie540 Chemistry & allied sciencesinstitution:unirostockinstitution:unirostockUniversität RostockUniversity of RostockUniversität RostockUniversität RostockUni.Rostockhttp://d-nb.info/gnd/38329-6institution:unirostock.mnfinstitution:unirostock.mnfMathematisch-Naturwissenschaftliche FakultätFaculty of Mathematics and Natural SciencesUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätMathematisch-Natur-<br />wissenschaftliche FakultätUni.Rostock.Fakultaet.MNFhttp://d-nb.info/gnd/2147083-2licenseinfo:worklicenseinfo:workWerkworklicenseinfo:work.rightsreservedlicenseinfo:work.rightsreservedalle Rechte vorbehaltenall rights reserved/creativecommons/r/reserved/0.9/88x31.png[DE-28]Urheberrechtsschutz 1.0$gRights Statements$uhttp://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/licenseinfo:depositlicenseinfo:depositVeröffentlichungsgenehmigungpermission to storelicenseinfo:deposit.rightsgrantedlicenseinfo:deposit.rightsgrantedNutzungsrechte erteiltrights grantedlicenseinfo:metadatalicenseinfo:metadataLizenzen für Metadatenlicenseinfo:metadata.cc0licenseinfo:metadata.cc0Lizenz Metadaten: CC0license metadata: CC0/creativecommons/p/zero/1.0/88x31.pnghttps://creativecommons.org/publicdomain/zero/1.0/accesscondition:openaccessaccesscondition:openaccessfrei zugänglich (Open Access)open accesshttp://purl.org/coar/access_right/c_abf2OAfreeinfo:eu-repo/semantics/openAccess[DE-28]Open Access$gControlled Vocabulary for Access Rights$uhttp://purl.org/coar/access_right/c_abf2rfc5646:enrfc5646:enEnglischEnglishengengCopper catalyzed sun fuel generation by CO2 and H2O reductionCopper catalyzed sun fuel generation by CO2 and H2O reductiongnd:1202554695gnd:112081908orcid:0000-0001-5709-0965gnd:136437524gnd:38329-6gnd:2147083-2gnd:1202554695gnd:112081908orcid:0000-0001-5709-0965gnd:136437524gnd:38329-6gnd:2147083-2rosdok_disshab_0000002221-d4103035e52gnd:1202554695Stefanie KreftStefanie Kreftrosdok_disshab_0000002221-d4103035e66gnd:112081908orcid:0000-0001-5709-0965Matthias BellerMatthias Bellerrosdok_disshab_0000002221-d4103035e82gnd:136437524Ralf LudwigRalf Ludwigrosdok_disshab_0000002221-d4103035e96gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000002221-d4103035e108gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätStefanie KreftMatthias BellerRalf LudwigUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätStefanie KreftMatthias BellerRalf LudwigUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätStefanie KreftRostockUniversität Rostockepub.dissertationhttp://purl.uni-rostock.de/rosdok/id00002594urn:nbn:de:gbv:28-rosdok_id00002594-810.18453/rosdok_id00002594FotokatalyseReduktionEnergieerzeugungKatalysatorHeterogeneous copper-based catalysts have been investigated for the photocatalytic H2O and CO2 reduction. Ex situ and in situ synthesized catalysts supported on inert silica have been developed for the photocatalytic proton reduction. The best supported photocatalyst achieved a significantly higher activity compared to the initial homogeneous precursor. In a second project highly porous photocatalysts have been synthesized, applied in aqueous CO2 reduction and characterized by in situ XAS, EPR and UV-vis measurements. An improved catalytic performance was observed by the addition of oxygen.20192019Matthias Beller (Universität Rostock, Leibniz-Institut für Katalyse e.V.) ; Ralf Ludwig (Universität Rostock, Institut für Chemie)Enthält Zeitschriftenartikelvorgelegt von Stefanie Kreftepub.dissertation1 Kreft_Dissertation_2020.pdf 15016103 7e32251ffa56136cc3d2c0987322aa2f rosdok/id000025941687013330Oau2020-01-102023-08-05T19:13:53ZrdaConverted from PICA to MODS using Pica2Mods XSLT Transformer 2.7 [SCM: "0c0e7a3c226a4a0cbcbec39b493c3c5257339ab8" "v2.7" "2023-08-04T00:00:00+0200"] with mode 'DEFAULT'.DissertationHochschulschriftCopper catalyzed sun fuel generation by CO2 and H2O reductionHeterogeneous copper-based catalysts have been investigated for the photocatalytic H2O and CO2 reduction. Ex situ and in situ synthesized catalysts supported on inert silica have been developed for the photocatalytic proton reduction. The best supported photocatalyst achieved a significantly higher activity compared to the initial homogeneous precursor. In a second project highly porous photocatalysts have been synthesized, applied in aqueous CO2 reduction and characterized by in situ XAS, EPR and UV-vis measurements. 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Ex situ and in situ synthesized catalysts supported on inert silica have been developed for the photocatalytic proton reduction. The best supported photocatalyst achieved a significantly higher activity compared to the initial homogeneous precursor. In a second project highly porous photocatalysts have been synthesized, applied in aqueous CO2 reduction and characterized by in situ XAS, EPR and UV-vis measurements. An improved catalytic performance was observed by the addition of oxygen.20192019Matthias Beller (Universität Rostock, Leibniz-Institut für Katalyse e.V.) ; Ralf Ludwig (Universität Rostock, Institut für Chemie)Enthält Zeitschriftenartikelvorgelegt von Stefanie Kreft[xslt]Saxonrosdok/id00002594https://purl.uni-rostock.de/rosdok/id00002594168701333010.18453/rosdok_id00002594urn:nbn:de:gbv:28-rosdok_id00002594-8Stefanie KreftKreft StefanieCopper catalyzed sun fuel generation by CO2 and H2O reductionDissertationdoctoral thesisUniversität Rostock, 2019Heterogeneous copper-based catalysts have been investigated for the photocatalytic H2O and CO2 reduction. Ex situ and in situ synthesized catalysts supported on inert silica have been developed for the photocatalytic proton reduction. The best supported photocatalyst achieved a significantly higher…Stefanie KreftCopper catalyzed sun fuel generation by CO2 and H2O reductionUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00002594StefanieKreft1985 -VerfasserInaut1202554695MatthiasBeller1962 -AkademischeR BetreuerIndgs1120819080000-0001-5709-0965RalfLudwig1961 -AkademischeR BetreuerIndgs13643752438329-6Universität Rostock1419 -Grad-verleihende Institutiondgg2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg[purl]http://purl.uni-rostock.de/rosdok/id00002594[urn]urn:nbn:de:gbv:28-rosdok_id00002594-8[doi]10.18453/rosdok_id00002594open_access20192019epoch:21th_centuryrfc5646:endoctype:epub.dissertationaccesscondition:openaccessSDNB:540institution:unirostock.mnfstate:published