mycoreobjectrosdok_disshab_0000002779rosdok_disshab_0000002779rosdokdisshabrosdok_derivate_00001983252023-08-08T10:14:20.562Z2022-07-13T14:09:43.954ZadministratoreditorMSpublished1rosdok_derivate_0000198325truetruederivate_types:fulltextVolltextfulltextwf_edit_epub wf_register_epubstate:publishedstate:publishedveröffentlichtpublishedrosdok/id000037791810124166Oau2022-07-132023-08-05T19:20:30ZrdaConverted from PICA to MODS using Pica2Mods XSLT Transformer 2.7 [SCM: "0c0e7a3c226a4a0cbcbec39b493c3c5257339ab8" "v2.7" "2023-08-04T00:00:00+0200"] with mode 'DEFAULT'.DissertationHochschulschriftUnraveling property-performance relationships in CO2 hydrogenation over iron-based catalystsThis thesis deals with the development of iron-based catalysts for CO2 hydrogenation to higher hydrocarbons and understanding of fundamentals relevant for activity and selectivity. The most decisive factors affecting activity and selectivity were identified by statistical approaches. The promotion effects of alkali metal promoter on CO2 hydrogenation over Fe-based catalysts were elucidated through characterization and kinetic analyses. This thesis also contributes to understanding of the interplay between physicochemical properties of promoter-free Fe-based catalyst and catalytic performance.QingxinYang1993 -VerfasserInaut1262432138Evgenii V.KondratenkoAkademischeR BetreuerIndgs11065657890000-0003-0431-6937AndreiKhodakovAkademischeR BetreuerIndgsUniversität Lille38329-6Universität Rostock1419 -Grad-verleihende Institutiondgg2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttp://purl.uni-rostock.de/rosdok/id00003779urn:nbn:de:gbv:28-rosdok_id00003779-610.18453/rosdok_id00003779540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en2022Universität RostockRostockmonographic202220222022Universitätsbibliothek RostockRostock2022Universitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00003779Evgenii Kondratenko (Leibniz-Institut für Katalyse e.V.) ; Andrei Khodakov (Universität Lille)[{"affil":"Leibniz-Institut für Katalyse e.V.","name":"Kondratenko, Evgenii"},{"affil":"Universität Lille","name":"Khodakov, Andrei"}]vorgelegt von Qingxin YangKatalysatorHydrierungKohlendioxidLeibniz-Institut für Katalyse e.V.Kondratenko, EvgeniiUniversität LilleKhodakov, Andreidoctype:epubdoctype:epubDokumenttypDocument typedoctype:epub.dissertationdoctype:epub.dissertationDissertationdoctoral thesisdiniPublType:doctoralThesis diniPublType2022:PhDThesis XMetaDissPlusThesisLevel:thesis.doctoralinfo:eu-repo/semantics/doctoralThesisdocumentnatureOfContent:ppn_105825778natureOfContent:ppn_105825778HochschulschriftdiniPublType2022:DoctoralThesisdiniPublType2022:DoctoralThesisDissertation oder HabilitationDoctoral thesisDRIVERdiniPublType2022:PhDThesisdiniPublType2022:PhDThesisDissertationPhD thesisKDSF (Pu34)XMetaDissPlusThesisLevel:thesis.doctoralXMetaDissPlusThesisLevel:thesis.doctoralDoktorarbeitdoctoral thesisSDNB:540SDNB:540540 Chemie540 Chemistry & allied sciencesinstitution:unirostockinstitution:unirostockUniversität RostockUniversity of RostockUniversität RostockUniversität RostockUni.Rostockhttp://d-nb.info/gnd/38329-6institution:unirostock.mnfinstitution:unirostock.mnfMathematisch-Naturwissenschaftliche FakultätFaculty of Mathematics and Natural SciencesUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätMathematisch-Natur-<br />wissenschaftliche FakultätUni.Rostock.Fakultaet.MNFhttp://d-nb.info/gnd/2147083-2licenseinfo:worklicenseinfo:workWerkworklicenseinfo:work.rightsreservedlicenseinfo:work.rightsreservedalle Rechte vorbehaltenall rights reserved/creativecommons/r/reserved/0.9/88x31.png[DE-28]Urheberrechtsschutz 1.0$gRights Statements$uhttp://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/licenseinfo:depositlicenseinfo:depositVeröffentlichungsgenehmigungpermission to storelicenseinfo:deposit.rightsgrantedlicenseinfo:deposit.rightsgrantedNutzungsrechte erteiltrights grantedlicenseinfo:metadatalicenseinfo:metadataLizenzen für Metadatenlicenseinfo:metadata.cc0licenseinfo:metadata.cc0Lizenz Metadaten: CC0license metadata: CC0/creativecommons/p/zero/1.0/88x31.pnghttps://creativecommons.org/publicdomain/zero/1.0/accesscondition:openaccessaccesscondition:openaccessfrei zugänglich (Open Access)open accesshttp://purl.org/coar/access_right/c_abf2OAfreeinfo:eu-repo/semantics/openAccess[DE-28]Open Access$gControlled Vocabulary for Access Rights$uhttp://purl.org/coar/access_right/c_abf2rfc5646:enrfc5646:enEnglischEnglishengengUnraveling property-performance relationships in CO2 hydrogenation over iron-based catalystsUnraveling property-performance relationships in CO2 hydrogenation over iron-based catalystsgnd:1262432138gnd:1106565789orcid:0000-0003-0431-6937gnd:38329-6gnd:2147083-2gnd:1262432138gnd:1106565789orcid:0000-0003-0431-6937gnd:38329-6gnd:2147083-2rosdok_disshab_0000002779-d1669552e52gnd:1262432138Qingxin YangQingxin Yangrosdok_disshab_0000002779-d1669552e66gnd:1106565789orcid:0000-0003-0431-6937Evgenii V. KondratenkoEvgenii V. Kondratenkorosdok_disshab_0000002779-d1669552e80Andrei KhodakovAndrei Khodakovrosdok_disshab_0000002779-d1669552e91gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000002779-d1669552e103gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätQingxin YangEvgenii V. KondratenkoAndrei KhodakovUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätQingxin YangEvgenii V. KondratenkoAndrei KhodakovUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätQingxin YangRostockUniversität Rostockepub.dissertationhttp://purl.uni-rostock.de/rosdok/id00003779urn:nbn:de:gbv:28-rosdok_id00003779-610.18453/rosdok_id00003779KatalysatorHydrierungKohlendioxidThis thesis deals with the development of iron-based catalysts for CO2 hydrogenation to higher hydrocarbons and understanding of fundamentals relevant for activity and selectivity. The most decisive factors affecting activity and selectivity were identified by statistical approaches. The promotion effects of alkali metal promoter on CO2 hydrogenation over Fe-based catalysts were elucidated through characterization and kinetic analyses. This thesis also contributes to understanding of the interplay between physicochemical properties of promoter-free Fe-based catalyst and catalytic performance.20222022Evgenii Kondratenko (Leibniz-Institut für Katalyse e.V.) ; Andrei Khodakov (Universität Lille)[{"affil":"Leibniz-Institut für Katalyse e.V.","name":"Kondratenko, Evgenii"},{"affil":"Universität Lille","name":"Khodakov, Andrei"}]vorgelegt von Qingxin Yangepub.dissertation1 Yang_Dissertation_2022.pdf 26357524 121e4f2b1e21fcbfaa623dafbb8a0451 rosdok/id000037791810124166Oau2022-07-132023-08-05T19:20:30ZrdaConverted from PICA to MODS using Pica2Mods XSLT Transformer 2.7 [SCM: "0c0e7a3c226a4a0cbcbec39b493c3c5257339ab8" "v2.7" "2023-08-04T00:00:00+0200"] with mode 'DEFAULT'.DissertationHochschulschriftUnraveling property-performance relationships in CO2 hydrogenation over iron-based catalystsThis thesis deals with the development of iron-based catalysts for CO2 hydrogenation to higher hydrocarbons and understanding of fundamentals relevant for activity and selectivity. The most decisive factors affecting activity and selectivity were identified by statistical approaches. The promotion effects of alkali metal promoter on CO2 hydrogenation over Fe-based catalysts were elucidated through characterization and kinetic analyses. This thesis also contributes to understanding of the interplay between physicochemical properties of promoter-free Fe-based catalyst and catalytic performance.QingxinYang1993 -VerfasserInaut1262432138Evgenii V.KondratenkoAkademischeR BetreuerIndgs11065657890000-0003-0431-6937AndreiKhodakovAkademischeR BetreuerIndgsUniversität Lille38329-6Universität Rostock1419 -Grad-verleihende Institutiondgg2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttp://purl.uni-rostock.de/rosdok/id00003779urn:nbn:de:gbv:28-rosdok_id00003779-610.18453/rosdok_id00003779540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en2022Universität RostockRostockmonographic202220222022Universitätsbibliothek RostockRostock2022Universitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00003779Evgenii Kondratenko (Leibniz-Institut für Katalyse e.V.) ; Andrei Khodakov (Universität Lille)[{"affil":"Leibniz-Institut für Katalyse e.V.","name":"Kondratenko, Evgenii"},{"affil":"Universität Lille","name":"Khodakov, Andrei"}]vorgelegt von Qingxin YangKatalysatorHydrierungKohlendioxid Leibniz-Institut für Katalyse e.V. Kondratenko, Evgenii Universität Lille Khodakov, Andrei 2022-07-13T14:09:43.954Z 2023-08-08T10:14:20.562Z 2023-08-18T10:14:20.567Z {"identifier":"rosdok/id00003779","type":"local_id","additional":"","service":"MCRLocalID","created":"2022-07-13T14:09:43.980Z","registered":"2022-07-13T14:09:43.980Z"} editorMS {"identifier":"urn:nbn:de:gbv:28-rosdok_id00003779-6","type":"dnbUrn","additional":"","service":"RosDokURN","created":"2022-07-13T14:09:43.987Z","registered":"2022-07-13T18:48:32.390Z"} administratorfulltextfile/rosdok_disshab_0000002779/rosdok_derivate_0000198325/Yang_Dissertation_2022.pdfUnraveling property-performance relationships in CO2 hydrogenation over iron-based catalystsUnraveling property-performance relationships in CO2 hydrogenation over iron-based catalystsgnd:1262432138gnd:1106565789orcid:0000-0003-0431-6937gnd:38329-6gnd:2147083-2gnd:1262432138gnd:1106565789orcid:0000-0003-0431-6937gnd:38329-6gnd:2147083-2rosdok_disshab_0000002779-d1669552e52gnd:1262432138Qingxin YangQingxin Yangrosdok_disshab_0000002779-d1669552e66gnd:1106565789orcid:0000-0003-0431-6937Evgenii V. KondratenkoEvgenii V. Kondratenkorosdok_disshab_0000002779-d1669552e80Andrei KhodakovAndrei Khodakovrosdok_disshab_0000002779-d1669552e91gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000002779-d1669552e103gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätQingxin YangEvgenii V. KondratenkoAndrei KhodakovUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätQingxin YangEvgenii V. KondratenkoAndrei KhodakovUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätQingxin YangRostockUniversität Rostockepub.dissertationhttp://purl.uni-rostock.de/rosdok/id00003779urn:nbn:de:gbv:28-rosdok_id00003779-610.18453/rosdok_id00003779KatalysatorHydrierungKohlendioxidThis thesis deals with the development of iron-based catalysts for CO2 hydrogenation to higher hydrocarbons and understanding of fundamentals relevant for activity and selectivity. The most decisive factors affecting activity and selectivity were identified by statistical approaches. The promotion effects of alkali metal promoter on CO2 hydrogenation over Fe-based catalysts were elucidated through characterization and kinetic analyses. This thesis also contributes to understanding of the interplay between physicochemical properties of promoter-free Fe-based catalyst and catalytic performance.20222022Evgenii Kondratenko (Leibniz-Institut für Katalyse e.V.) ; Andrei Khodakov (Universität Lille)[{"affil":"Leibniz-Institut für Katalyse e.V.","name":"Kondratenko, Evgenii"},{"affil":"Universität Lille","name":"Khodakov, Andrei"}]vorgelegt von Qingxin Yang[xslt]Saxonrosdok/id00003779https://purl.uni-rostock.de/rosdok/id00003779181012416610.18453/rosdok_id00003779urn:nbn:de:gbv:28-rosdok_id00003779-6Qingxin YangYang QingxinUnraveling property-performance relationships in CO2 hydrogenation over iron-based catalystsDissertationdoctoral thesisUniversität Rostock, 2022This thesis deals with the development of iron-based catalysts for CO2 hydrogenation to higher hydrocarbons and understanding of fundamentals relevant for activity and selectivity. The most decisive factors affecting activity and selectivity were identified by statistical approaches. The promotion…Qingxin YangUnraveling property-performance relationships in CO2 hydrogenation over iron-based catalystsUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00003779QingxinYang1993 -VerfasserInaut1262432138Evgenii V.KondratenkoAkademischeR BetreuerIndgs11065657890000-0003-0431-6937AndreiKhodakovAkademischeR BetreuerIndgsUniversität Lille38329-6Universität Rostock1419 -Grad-verleihende Institutiondgg2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg[purl]http://purl.uni-rostock.de/rosdok/id00003779[urn]urn:nbn:de:gbv:28-rosdok_id00003779-6[doi]10.18453/rosdok_id00003779open_access20222022epoch:21th_centuryrfc5646:endoctype:epub.dissertationaccesscondition:openaccessSDNB:540institution:unirostock.mnfstate:published