mycoreobjectrosdok_disshab_0000002859rosdok_disshab_0000002859rosdokdisshabrosdok_derivate_00002028462023-08-08T10:14:50.885Z2022-12-15T08:47:59.694ZadministratoreditorMSpublished1rosdok_derivate_0000202846truetruederivate_types:fulltextVolltextfulltextwf_edit_epub wf_register_epubstate:publishedstate:publishedveröffentlichtpublishedrosdok/id000040581827169001Oau2022-12-152023-08-05T19:21:36ZrdaConverted from PICA to MODS using Pica2Mods XSLT Transformer 2.7 [SCM: "0c0e7a3c226a4a0cbcbec39b493c3c5257339ab8" "v2.7" "2023-08-04T00:00:00+0200"] with mode 'DEFAULT'.DissertationHochschulschriftValue-added products from bio-based platform chemicalsThis thesis describes the use of platform-derived chemicals as novel, bio-based intermediates to the synthesis of value-added compounds. Levulinic acid-derived angelica lactones were used to preapre C3 chemicals such as malonic acid via ozonolysis and novel poly-norbornene-like polymers. Glycolaldehyde, obtained from lignocellulose, was employed for the first time as C1 building block for the N-formylation of secondary amines by catalyst-free radical oxidation. Methyl vinyl glycolate, a side stream product of the production of lactate from sugars, was used as precursor for bio-based polyester.AndreaDell'Acqua1994 -VerfasserInaut12756178750000-0003-1546-0045Johannes G.Vriesde1951 -AkademischeR BetreuerIndgs132252880Gert-JanGruterAkademischeR BetreuerIndgsFaculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam38329-6Universität Rostock1419 -Grad-verleihende Institutiondgg2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttp://purl.uni-rostock.de/rosdok/id00004058urn:nbn:de:gbv:28-rosdok_id00004058-010.18453/rosdok_id00004058540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en2022Universität RostockRostockmonographic202220222022Universitätsbibliothek RostockRostock2022Universitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00004058Enthält ZeitschriftenartikelJohannes G. de Vries (Leibniz-Institut für Katalyse e. V., Rostock) ; Gert-Jan Gruter (Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam)[{"affil":"Leibniz-Institut für Katalyse e. V., Rostock","name":"de Vries, Johannes G."},{"affil":"Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam","name":"Gruter, Gert-Jan"}]vorgelegt von Andrea Dell'AcquaKohlenhydrateLävulinsäureGlykolaldehydPolymereMonomereLeibniz-Institut für Katalyse e. V., Rostockde Vries, Johannes G.Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of AmsterdamGruter, Gert-Jandoctype:epubdoctype:epubDokumenttypDocument typedoctype:epub.dissertationdoctype:epub.dissertationDissertationdoctoral thesisdiniPublType:doctoralThesis diniPublType2022:PhDThesis XMetaDissPlusThesisLevel:thesis.doctoralinfo:eu-repo/semantics/doctoralThesisdocumentnatureOfContent:ppn_105825778natureOfContent:ppn_105825778HochschulschriftdiniPublType2022:DoctoralThesisdiniPublType2022:DoctoralThesisDissertation oder HabilitationDoctoral thesisDRIVERdiniPublType2022:PhDThesisdiniPublType2022:PhDThesisDissertationPhD thesisKDSF (Pu34)XMetaDissPlusThesisLevel:thesis.doctoralXMetaDissPlusThesisLevel:thesis.doctoralDoktorarbeitdoctoral thesisSDNB:540SDNB:540540 Chemie540 Chemistry & allied sciencesinstitution:unirostockinstitution:unirostockUniversität RostockUniversity of RostockUniversität RostockUniversität RostockUni.Rostockhttp://d-nb.info/gnd/38329-6institution:unirostock.mnfinstitution:unirostock.mnfMathematisch-Naturwissenschaftliche FakultätFaculty of Mathematics and Natural SciencesUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätMathematisch-Natur-<br />wissenschaftliche FakultätUni.Rostock.Fakultaet.MNFhttp://d-nb.info/gnd/2147083-2licenseinfo:worklicenseinfo:workWerkworklicenseinfo:work.rightsreservedlicenseinfo:work.rightsreservedalle Rechte vorbehaltenall rights reserved/creativecommons/r/reserved/0.9/88x31.png[DE-28]Urheberrechtsschutz 1.0$gRights Statements$uhttp://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/licenseinfo:depositlicenseinfo:depositVeröffentlichungsgenehmigungpermission to storelicenseinfo:deposit.rightsgrantedlicenseinfo:deposit.rightsgrantedNutzungsrechte erteiltrights grantedlicenseinfo:metadatalicenseinfo:metadataLizenzen für Metadatenlicenseinfo:metadata.cc0licenseinfo:metadata.cc0Lizenz Metadaten: CC0license metadata: CC0/creativecommons/p/zero/1.0/88x31.pnghttps://creativecommons.org/publicdomain/zero/1.0/accesscondition:openaccessaccesscondition:openaccessfrei zugänglich (Open Access)open accesshttp://purl.org/coar/access_right/c_abf2OAfreeinfo:eu-repo/semantics/openAccess[DE-28]Open Access$gControlled Vocabulary for Access Rights$uhttp://purl.org/coar/access_right/c_abf2rfc5646:enrfc5646:enEnglischEnglishengengValue-added products from bio-based platform chemicalsValue-added products from bio-based platform chemicalsgnd:1275617875orcid:0000-0003-1546-0045gnd:132252880gnd:38329-6gnd:2147083-2gnd:1275617875orcid:0000-0003-1546-0045gnd:132252880gnd:38329-6gnd:2147083-2rosdok_disshab_0000002859-d2170025e52gnd:1275617875orcid:0000-0003-1546-0045Andrea Dell'AcquaAndrea Dell'Acquarosdok_disshab_0000002859-d2170025e68gnd:132252880Johannes G. Vries deJohannes G. Vries derosdok_disshab_0000002859-d2170025e84Gert-Jan GruterGert-Jan Gruterrosdok_disshab_0000002859-d2170025e95gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000002859-d2170025e107gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätAndrea Dell'AcquaJohannes G. Vries deGert-Jan GruterUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätAndrea Dell'AcquaJohannes G. Vries deGert-Jan GruterUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätAndrea Dell'AcquaRostockUniversität Rostockepub.dissertationhttp://purl.uni-rostock.de/rosdok/id00004058urn:nbn:de:gbv:28-rosdok_id00004058-010.18453/rosdok_id00004058KohlenhydrateLävulinsäureGlykolaldehydPolymereMonomereThis thesis describes the use of platform-derived chemicals as novel, bio-based intermediates to the synthesis of value-added compounds. Levulinic acid-derived angelica lactones were used to preapre C3 chemicals such as malonic acid via ozonolysis and novel poly-norbornene-like polymers. Glycolaldehyde, obtained from lignocellulose, was employed for the first time as C1 building block for the N-formylation of secondary amines by catalyst-free radical oxidation. Methyl vinyl glycolate, a side stream product of the production of lactate from sugars, was used as precursor for bio-based polyester.20222022Enthält ZeitschriftenartikelJohannes G. de Vries (Leibniz-Institut für Katalyse e. V., Rostock) ; Gert-Jan Gruter (Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam)[{"affil":"Leibniz-Institut für Katalyse e. V., Rostock","name":"de Vries, Johannes G."},{"affil":"Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam","name":"Gruter, Gert-Jan"}]vorgelegt von Andrea Dell'Acquaepub.dissertation1 DellAcqua_Dissertation_2022.pdf 14289090 b049a5e0f8e72e5cf9158aa000e2c3eb rosdok/id000040581827169001Oau2022-12-152023-08-05T19:21:36ZrdaConverted from PICA to MODS using Pica2Mods XSLT Transformer 2.7 [SCM: "0c0e7a3c226a4a0cbcbec39b493c3c5257339ab8" "v2.7" "2023-08-04T00:00:00+0200"] with mode 'DEFAULT'.DissertationHochschulschriftValue-added products from bio-based platform chemicalsThis thesis describes the use of platform-derived chemicals as novel, bio-based intermediates to the synthesis of value-added compounds. Levulinic acid-derived angelica lactones were used to preapre C3 chemicals such as malonic acid via ozonolysis and novel poly-norbornene-like polymers. Glycolaldehyde, obtained from lignocellulose, was employed for the first time as C1 building block for the N-formylation of secondary amines by catalyst-free radical oxidation. Methyl vinyl glycolate, a side stream product of the production of lactate from sugars, was used as precursor for bio-based polyester.AndreaDell'Acqua1994 -VerfasserInaut12756178750000-0003-1546-0045Johannes G.Vriesde1951 -AkademischeR BetreuerIndgs132252880Gert-JanGruterAkademischeR BetreuerIndgsFaculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam38329-6Universität Rostock1419 -Grad-verleihende Institutiondgg2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttp://purl.uni-rostock.de/rosdok/id00004058urn:nbn:de:gbv:28-rosdok_id00004058-010.18453/rosdok_id00004058540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en2022Universität RostockRostockmonographic202220222022Universitätsbibliothek RostockRostock2022Universitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00004058Enthält ZeitschriftenartikelJohannes G. de Vries (Leibniz-Institut für Katalyse e. V., Rostock) ; Gert-Jan Gruter (Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam)[{"affil":"Leibniz-Institut für Katalyse e. V., Rostock","name":"de Vries, Johannes G."},{"affil":"Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam","name":"Gruter, Gert-Jan"}]vorgelegt von Andrea Dell'AcquaKohlenhydrateLävulinsäureGlykolaldehydPolymereMonomere Leibniz-Institut für Katalyse e. V., Rostock de Vries, Johannes G. Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam Gruter, Gert-Jan 2022-12-15T08:47:59.694Z 2023-08-08T10:14:50.885Z 2023-08-18T10:14:50.890Z {"identifier":"rosdok/id00004058","type":"local_id","additional":"","service":"MCRLocalID","created":"2022-12-15T08:47:59.712Z","registered":"2022-12-15T08:47:59.712Z"} editorMS {"identifier":"urn:nbn:de:gbv:28-rosdok_id00004058-0","type":"dnbUrn","additional":"","service":"RosDokURN","created":"2022-12-15T08:47:59.718Z","registered":"2022-12-15T20:00:31.433Z"} administratorfulltextfile/rosdok_disshab_0000002859/rosdok_derivate_0000202846/DellAcqua_Dissertation_2022.pdfValue-added products from bio-based platform chemicalsValue-added products from bio-based platform chemicalsgnd:1275617875orcid:0000-0003-1546-0045gnd:132252880gnd:38329-6gnd:2147083-2gnd:1275617875orcid:0000-0003-1546-0045gnd:132252880gnd:38329-6gnd:2147083-2rosdok_disshab_0000002859-d2170025e52gnd:1275617875orcid:0000-0003-1546-0045Andrea Dell'AcquaAndrea Dell'Acquarosdok_disshab_0000002859-d2170025e68gnd:132252880Johannes G. Vries deJohannes G. Vries derosdok_disshab_0000002859-d2170025e84Gert-Jan GruterGert-Jan Gruterrosdok_disshab_0000002859-d2170025e95gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000002859-d2170025e107gnd:2147083-2Universität Rostock Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätAndrea Dell'AcquaJohannes G. Vries deGert-Jan GruterUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätAndrea Dell'AcquaJohannes G. Vries deGert-Jan GruterUniversität RostockUniversität Rostock Mathematisch-Naturwissenschaftliche FakultätAndrea Dell'AcquaRostockUniversität Rostockepub.dissertationhttp://purl.uni-rostock.de/rosdok/id00004058urn:nbn:de:gbv:28-rosdok_id00004058-010.18453/rosdok_id00004058KohlenhydrateLävulinsäureGlykolaldehydPolymereMonomereThis thesis describes the use of platform-derived chemicals as novel, bio-based intermediates to the synthesis of value-added compounds. Levulinic acid-derived angelica lactones were used to preapre C3 chemicals such as malonic acid via ozonolysis and novel poly-norbornene-like polymers. Glycolaldehyde, obtained from lignocellulose, was employed for the first time as C1 building block for the N-formylation of secondary amines by catalyst-free radical oxidation. Methyl vinyl glycolate, a side stream product of the production of lactate from sugars, was used as precursor for bio-based polyester.20222022Enthält ZeitschriftenartikelJohannes G. de Vries (Leibniz-Institut für Katalyse e. V., Rostock) ; Gert-Jan Gruter (Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam)[{"affil":"Leibniz-Institut für Katalyse e. V., Rostock","name":"de Vries, Johannes G."},{"affil":"Faculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam","name":"Gruter, Gert-Jan"}]vorgelegt von Andrea Dell'Acqua[xslt]Saxonrosdok/id00004058https://purl.uni-rostock.de/rosdok/id00004058182716900110.18453/rosdok_id00004058urn:nbn:de:gbv:28-rosdok_id00004058-0Andrea Dell'AcquaDell'Acqua AndreaValue-added products from bio-based platform chemicalsDissertationdoctoral thesisUniversität Rostock, 2022This thesis describes the use of platform-derived chemicals as novel, bio-based intermediates to the synthesis of value-added compounds. Levulinic acid-derived angelica lactones were used to preapre C3 chemicals such as malonic acid via ozonolysis and novel poly-norbornene-like polymers.…Andrea Dell'AcquaValue-added products from bio-based platform chemicalsUniversitätsbibliothek Rostockhttp://purl.uni-rostock.de/rosdok/id00004058AndreaDell'Acqua1994 -VerfasserInaut12756178750000-0003-1546-0045Johannes G.Vriesde1951 -AkademischeR BetreuerIndgs132252880Gert-JanGruterAkademischeR BetreuerIndgsFaculty of Science Van 't Hoff Institute for Molecular Sciences, University of Amsterdam38329-6Universität Rostock1419 -Grad-verleihende Institutiondgg2147083-2Universität RostockMathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg[purl]http://purl.uni-rostock.de/rosdok/id00004058[urn]urn:nbn:de:gbv:28-rosdok_id00004058-0[doi]10.18453/rosdok_id00004058open_access20222022epoch:21th_centuryrfc5646:endoctype:epub.dissertationaccesscondition:openaccessSDNB:540institution:unirostock.mnfstate:published