mycoreobjectrosdok_disshab_0000003227rosdok_disshab_0000003227rosdokdisshabrosdok_derivate_00002235672025-02-28T11:00:02.809Z2025-02-27T15:52:23.195ZMCRJANITOReditorFGpublished1rosdok_derivate_0000223567truetruederivate_types:fulltextVolltextfulltextwf_edit_epub wf_register_epubstate:publishedstate:publishedveröffentlichtpublishedrosdok/id000047451918745048Oau2025-02-272025-02-27T16:01:48ZrdaConverted from PICA to MODS using Pica2MODS XSLT Transformer 2.10 [SCM: "f6c168af690edb7cb65ef34e4a2bf7f8714c5d38" "v2.10" "2024-03-28T14:43:08+0100"] with mode 'DEFAULT'.DissertationHochschulschriftThermal and photocatalytic C-C and C-N bond formation by atom-transfer radical additions and photocycloadditionsThe content of this thesis is presented in three parts. In the first part, the radical functionalisation of biomass-derived 5-chloromethylfurfural (CMF) was described. In the second part, visible light-mediated triplet-sensitized [2+2] and [3+2] photocycloadditions of 2-cyanochromone with several alkenes were demonstrated using Iridium photocatalyst. The last part describes the a photocatalytic one-pot dehydrogenative Aza Paternò-Büchi reaction of dihydroquinoxalinones with substituted styrenes and acrylonitriles for the synthesis of diverse functionalised azetidine derivatives.RajeshDasi1996 -VerfasserInaut1357991592MalteBrasholz1978 -AkademischeR BetreuerIndgs1339772180000-0001-8184-646XUniversität RostockRobertFrancke1982 -AkademischeR BetreuerIndgs12276253910000-0002-4998-1829Leibniz-Institut für Katalyse38329-6Universität Rostock1419 - 19761990 -Grad-verleihende Institutiondgg2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttps://purl.uni-rostock.de/rosdok/id00004745urn:nbn:de:gbv:28-rosdok_id00004745-810.18453/rosdok_id00004745500 Naturwissenschaften540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en1 Online-Ressource (110 Seiten)2023Universität RostockRostockmonographic202420232025Universitätsbibliothek RostockRostock2025Universitätsbibliothek Rostockhttps://purl.uni-rostock.de/rosdok/id00004745Enthält ZeitschriftenartikelMalte Brasholz (Universität Rostock) ; Robert Francke (Leibniz-Institut für Katalyse)[{"name":"Brasholz, Malte","affil":"Universität Rostock"},{"name":"Francke, Robert","affil":"Leibniz-Institut für Katalyse"}]Dissertation, Universität Rostock, 2024, Kumulative Dissertationvorgelegt von Rajesh DasiBrasholz, MalteUniversität RostockFrancke, RobertLeibniz-Institut für Katalysedoctype:epubdoctype:epubDokumenttypDocument typedoctype:epub.dissertationdoctype:epub.dissertationDissertationdoctoral thesisdiniPublType:doctoralThesis diniPublType2022:PhDThesis XMetaDissPlusThesisLevel:thesis.doctoralinfo:eu-repo/semantics/doctoralThesisdocumentnatureOfContent:ppn_105825778natureOfContent:ppn_105825778HochschulschriftdiniPublType2022:DoctoralThesisdiniPublType2022:DoctoralThesisDissertation oder HabilitationDoctoral thesisDRIVERdiniPublType2022:PhDThesisdiniPublType2022:PhDThesisDissertationPhD thesisKDSF (Pu34)XMetaDissPlusThesisLevel:thesis.doctoralXMetaDissPlusThesisLevel:thesis.doctoralDoktorarbeitdoctoral thesisSDNB:500SDNB:500500 Naturwissenschaften500 Natural sciencesSDNB:540SDNB:540540 Chemie540 Chemistry & allied sciencesinstitution:unirostockinstitution:unirostockUniversität RostockUniversity of RostockUniversität RostockUniversität RostockUni.Rostockhttp://d-nb.info/gnd/38329-6institution:unirostock.mnfinstitution:unirostock.mnfMathematisch-Naturwissenschaftliche FakultätFaculty of Mathematics and Natural SciencesUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätMathematisch-Natur-<br />wissenschaftliche FakultätUni.Rostock.Fakultaet.MNFhttp://d-nb.info/gnd/2147083-2licenseinfo:worklicenseinfo:workWerkworklicenseinfo:work.rightsreservedlicenseinfo:work.rightsreservedalle Rechte vorbehaltenall rights reserved/creativecommons/r/reserved/0.9/88x31.png[DE-28]Urheberrechtsschutz 1.0$gRights Statements$uhttp://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/licenseinfo:depositlicenseinfo:depositVeröffentlichungsgenehmigungpermission to storelicenseinfo:deposit.rightsgrantedlicenseinfo:deposit.rightsgrantedNutzungsrechte erteiltrights grantedlicenseinfo:metadatalicenseinfo:metadataLizenzen für Metadatenlicenseinfo:metadata.cc0licenseinfo:metadata.cc0Lizenz Metadaten: CC0license metadata: CC0/creativecommons/p/zero/1.0/88x31.pnghttps://creativecommons.org/publicdomain/zero/1.0/accesscondition:openaccessaccesscondition:openaccessfrei zugänglich (Open Access)open accesshttp://purl.org/coar/access_right/c_abf2OAfreeinfo:eu-repo/semantics/openAccess[DE-28]Open Access$gControlled Vocabulary for Access Rights$uhttp://purl.org/coar/access_right/c_abf2rfc5646:enrfc5646:enEnglischEnglishengengThermal and photocatalytic C-C and C-N bond formation by atom-transfer radical additions and photocycloadditionsThermal and photocatalytic C-C and C-N bond formation by atom-transfer radical additions and photocycloadditionsgnd:1357991592gnd:133977218orcid:0000-0001-8184-646Xgnd:1227625391orcid:0000-0002-4998-1829gnd:38329-6gnd:2147083-2gnd:1357991592gnd:133977218orcid:0000-0001-8184-646Xgnd:1227625391orcid:0000-0002-4998-1829gnd:38329-6gnd:2147083-2rosdok_disshab_0000003227-d2190478e52gnd:1357991592Rajesh DasiRajesh Dasirosdok_disshab_0000003227-d2190478e66gnd:133977218orcid:0000-0001-8184-646XMalte BrasholzMalte Brasholzrosdok_disshab_0000003227-d2190478e83gnd:1227625391orcid:0000-0002-4998-1829Robert FranckeRobert Franckerosdok_disshab_0000003227-d2190478e100gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000003227-d2190478e114gnd:2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätRajesh DasiMalte BrasholzRobert FranckeUniversität RostockUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätRajesh DasiMalte BrasholzRobert FranckeUniversität RostockUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätRajesh DasiRostockUniversität Rostockepub.dissertationhttps://purl.uni-rostock.de/rosdok/id00004745urn:nbn:de:gbv:28-rosdok_id00004745-810.18453/rosdok_id00004745The content of this thesis is presented in three parts. In the first part, the radical functionalisation of biomass-derived 5-chloromethylfurfural (CMF) was described. In the second part, visible light-mediated triplet-sensitized [2+2] and [3+2] photocycloadditions of 2-cyanochromone with several alkenes were demonstrated using Iridium photocatalyst. The last part describes the a photocatalytic one-pot dehydrogenative Aza Paternò-Büchi reaction of dihydroquinoxalinones with substituted styrenes and acrylonitriles for the synthesis of diverse functionalised azetidine derivatives.20232023Enthält ZeitschriftenartikelMalte Brasholz (Universität Rostock) ; Robert Francke (Leibniz-Institut für Katalyse)[{"name":"Brasholz, Malte","affil":"Universität Rostock"},{"name":"Francke, Robert","affil":"Leibniz-Institut für Katalyse"}]Dissertation, Universität Rostock, 2024, Kumulative Dissertationvorgelegt von Rajesh Dasiepub.dissertation1 Dasi_Dissertation_2025.pdf 15726366 b7066e26b62d460926aa23194312d7e9 rosdok/id000047451918745048Oau2025-02-272025-02-27T16:01:48ZrdaConverted from PICA to MODS using Pica2MODS XSLT Transformer 2.10 [SCM: "f6c168af690edb7cb65ef34e4a2bf7f8714c5d38" "v2.10" "2024-03-28T14:43:08+0100"] with mode 'DEFAULT'.DissertationHochschulschriftThermal and photocatalytic C-C and C-N bond formation by atom-transfer radical additions and photocycloadditionsThe content of this thesis is presented in three parts. In the first part, the radical functionalisation of biomass-derived 5-chloromethylfurfural (CMF) was described. In the second part, visible light-mediated triplet-sensitized [2+2] and [3+2] photocycloadditions of 2-cyanochromone with several alkenes were demonstrated using Iridium photocatalyst. The last part describes the a photocatalytic one-pot dehydrogenative Aza Paternò-Büchi reaction of dihydroquinoxalinones with substituted styrenes and acrylonitriles for the synthesis of diverse functionalised azetidine derivatives.RajeshDasi1996 -VerfasserInaut1357991592MalteBrasholz1978 -AkademischeR BetreuerIndgs1339772180000-0001-8184-646XUniversität RostockRobertFrancke1982 -AkademischeR BetreuerIndgs12276253910000-0002-4998-1829Leibniz-Institut für Katalyse38329-6Universität Rostock1419 - 19761990 -Grad-verleihende Institutiondgg2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttps://purl.uni-rostock.de/rosdok/id00004745urn:nbn:de:gbv:28-rosdok_id00004745-810.18453/rosdok_id00004745500 Naturwissenschaften540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en1 Online-Ressource (110 Seiten)2023Universität RostockRostockmonographic202420232025Universitätsbibliothek RostockRostock2025Universitätsbibliothek Rostockhttps://purl.uni-rostock.de/rosdok/id00004745Enthält ZeitschriftenartikelMalte Brasholz (Universität Rostock) ; Robert Francke (Leibniz-Institut für Katalyse)[{"name":"Brasholz, Malte","affil":"Universität Rostock"},{"name":"Francke, Robert","affil":"Leibniz-Institut für Katalyse"}]Dissertation, Universität Rostock, 2024, Kumulative Dissertationvorgelegt von Rajesh Dasi Brasholz, Malte Universität Rostock Francke, Robert Leibniz-Institut für Katalyse 2025-02-27T15:52:23.195Z 2025-02-28T11:00:02.809Z 2025-03-10T11:00:02.827Z editorFG {"identifier":"rosdok/id00004745","type":"local_id","additional":"","service":"MCRLocalID","created":"2025-02-27T15:52:24.302Z"} {"identifier":"https://purl.uni-rostock.de/rosdok/id00004745","type":"purl","additional":"","service":"RosDokPURL","created":"2025-02-27T15:52:24.438Z","registrationStarted":"2025-02-27T16:43:27.725Z"} {"identifier":"10.18453/rosdok_id00004745","type":"doi","additional":"","service":"RosDokDOI","created":"2025-02-27T15:52:24.445Z","registrationStarted":"2025-02-27T16:43:27.425Z","registered":"2025-02-27T16:43:29.076Z"} {"identifier":"urn:nbn:de:gbv:28-rosdok_id00004745-8","type":"dnbUrn","additional":"","service":"RosDokURN","created":"2025-02-27T15:52:24.428Z","registered":"2025-02-28T09:28:04.343Z"} MCRJANITORfulltextfile/rosdok_disshab_0000003227/rosdok_derivate_0000223567/Dasi_Dissertation_2025.pdfThermal and photocatalytic C-C and C-N bond formation by atom-transfer radical additions and photocycloadditionsThermal and photocatalytic C-C and C-N bond formation by atom-transfer radical additions and photocycloadditionsgnd:1357991592gnd:133977218orcid:0000-0001-8184-646Xgnd:1227625391orcid:0000-0002-4998-1829gnd:38329-6gnd:2147083-2gnd:1357991592gnd:133977218orcid:0000-0001-8184-646Xgnd:1227625391orcid:0000-0002-4998-1829gnd:38329-6gnd:2147083-2rosdok_disshab_0000003227-d2190478e52gnd:1357991592Rajesh DasiRajesh Dasirosdok_disshab_0000003227-d2190478e66gnd:133977218orcid:0000-0001-8184-646XMalte BrasholzMalte Brasholzrosdok_disshab_0000003227-d2190478e83gnd:1227625391orcid:0000-0002-4998-1829Robert FranckeRobert Franckerosdok_disshab_0000003227-d2190478e100gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000003227-d2190478e114gnd:2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätRajesh DasiMalte BrasholzRobert FranckeUniversität RostockUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätRajesh DasiMalte BrasholzRobert FranckeUniversität RostockUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätRajesh DasiRostockUniversität Rostockepub.dissertationhttps://purl.uni-rostock.de/rosdok/id00004745urn:nbn:de:gbv:28-rosdok_id00004745-810.18453/rosdok_id00004745The content of this thesis is presented in three parts. In the first part, the radical functionalisation of biomass-derived 5-chloromethylfurfural (CMF) was described. In the second part, visible light-mediated triplet-sensitized [2+2] and [3+2] photocycloadditions of 2-cyanochromone with several alkenes were demonstrated using Iridium photocatalyst. The last part describes the a photocatalytic one-pot dehydrogenative Aza Paternò-Büchi reaction of dihydroquinoxalinones with substituted styrenes and acrylonitriles for the synthesis of diverse functionalised azetidine derivatives.20232023Enthält ZeitschriftenartikelMalte Brasholz (Universität Rostock) ; Robert Francke (Leibniz-Institut für Katalyse)[{"name":"Brasholz, Malte","affil":"Universität Rostock"},{"name":"Francke, Robert","affil":"Leibniz-Institut für Katalyse"}]Dissertation, Universität Rostock, 2024, Kumulative Dissertationvorgelegt von Rajesh Dasi[xslt]Saxonrosdok/id00004745https://purl.uni-rostock.de/rosdok/id00004745191874504810.18453/rosdok_id00004745urn:nbn:de:gbv:28-rosdok_id00004745-8Rajesh DasiDasi RajeshThermal and photocatalytic C-C and C-N bond formation by atom-transfer radical additions and photocycloadditionsDissertationdoctoral thesisUniversität Rostock, 2023The content of this thesis is presented in three parts. In the first part, the radical functionalisation of biomass-derived 5-chloromethylfurfural (CMF) was described. In the second part, visible light-mediated triplet-sensitized [2+2] and [3+2] photocycloadditions of 2-cyanochromone with several…Rajesh DasiThermal and photocatalytic C-C and C-N bond formation by atom-transfer radical additions and photocycloadditionsUniversitätsbibliothek Rostockhttps://purl.uni-rostock.de/rosdok/id00004745RajeshDasi1996 -VerfasserInaut1357991592MalteBrasholz1978 -AkademischeR BetreuerIndgs1339772180000-0001-8184-646XUniversität RostockRobertFrancke1982 -AkademischeR BetreuerIndgs12276253910000-0002-4998-1829Leibniz-Institut für Katalyse38329-6Universität Rostock1419 - 19761990 -Grad-verleihende Institutiondgg2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg[purl]https://purl.uni-rostock.de/rosdok/id00004745[urn]urn:nbn:de:gbv:28-rosdok_id00004745-8[doi]10.18453/rosdok_id00004745open_access20232023epoch:21th_centuryrfc5646:endoctype:epub.dissertationaccesscondition:openaccessSDNB:500SDNB:540institution:unirostock.mnfstate:published