mycoreobjectrosdok_disshab_0000003249rosdok_disshab_0000003249rosdokdisshabrosdok_derivate_00002243282025-05-09T13:04:52.814Z2025-05-09T12:29:47.631ZMCRJANITOReditorFGpublished1rosdok_derivate_0000224328truetruederivate_types:fulltextVolltextfulltextwf_edit_epub wf_register_epubstate:publishedstate:publishedveröffentlichtpublishedrosdok/id000047761925256413Oau2025-05-092025-05-09T12:47:14ZrdaConverted from PICA to MODS using Pica2MODS XSLT Transformer 2.10 [SCM: "f6c168af690edb7cb65ef34e4a2bf7f8714c5d38" "v2.10" "2024-03-28T14:43:08+0100"] with mode 'DEFAULT'.DissertationHochschulschriftSimultaneous direct optimal controla versatile approach for steering quantum molecular dynamicsControlling molecular processes by shaped laser pulses is a long-standing goal in Molecular Physics and Chemistry. Here, we suggest a direct optimal control approach based on a simultaneous simulation and optimization paradigm. This approach uses automatic differentiation, offering as advantages final time and model parameter optimization, as well as a wide range of terms in the performance functional and constraints that could be easily implemented in a plug-and-play fashion. The advantages of this approach will be showcased for diverse molecular model systems.Alejandro RubenovichRamos Ramos1992 -VerfasserInaut13650999620009-0002-0922-1996OliverKühn1964 -AkademischeR BetreuerIndgs1410564870000-0002-5132-2961University of RostockJean ChristopheTremblayAkademischeR BetreuerIndgs11675323410000-0001-8021-7063University of Lorraine38329-6Universität Rostock1419 - 19761990 -Grad-verleihende Institutiondgg2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttps://purl.uni-rostock.de/rosdok/id00004776urn:nbn:de:gbv:28-rosdok_id00004776-510.18453/rosdok_id00004776530 Physik540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en1 Online-Ressource (V, 89 Seiten)202418. März 2024Universität RostockRostockmonographic20242025Universitätsbibliothek RostockRostock2025Universitätsbibliothek Rostockhttps://purl.uni-rostock.de/rosdok/id00004776Enthält ZeitschriftenartikelOliver Kühn (University of Rostock) ; Jean Christophe Tremblay (University of Lorraine)[{"name":"Kühn, Oliver","affil":"University of Rostock"},{"name":"Tremblay, Jean Christophe","affil":"University of Lorraine"}]Dissertation, Universität Rostock, 2024, Kumulative Dissertationvorgelegt von Alejandro Rubenovich Ramos RamosKühn, OliverUniversity of RostockTremblay, Jean ChristopheUniversity of Lorrainedoctype:epubdoctype:epubDokumenttypDocument typedoctype:epub.dissertationdoctype:epub.dissertationDissertationdoctoral thesisdiniPublType:doctoralThesis diniPublType2022:PhDThesis XMetaDissPlusThesisLevel:thesis.doctoralinfo:eu-repo/semantics/doctoralThesisdocumentnatureOfContent:ppn_105825778natureOfContent:ppn_105825778HochschulschriftdiniPublType2022:DoctoralThesisdiniPublType2022:DoctoralThesisDissertation oder HabilitationDoctoral thesisDRIVERdiniPublType2022:PhDThesisdiniPublType2022:PhDThesisDissertationPhD thesisKDSF (Pu34)XMetaDissPlusThesisLevel:thesis.doctoralXMetaDissPlusThesisLevel:thesis.doctoralDoktorarbeitdoctoral thesisSDNB:530SDNB:530530 Physik530 PhysicsSDNB:540SDNB:540540 Chemie540 Chemistry & allied sciencesinstitution:unirostockinstitution:unirostockUniversität RostockUniversity of RostockUniversität RostockUniversität RostockUni.Rostockhttp://d-nb.info/gnd/38329-6institution:unirostock.mnfinstitution:unirostock.mnfMathematisch-Naturwissenschaftliche FakultätFaculty of Mathematics and Natural SciencesUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätMathematisch-Natur-<br />wissenschaftliche FakultätUni.Rostock.Fakultaet.MNFhttp://d-nb.info/gnd/2147083-2licenseinfo:worklicenseinfo:workWerkworklicenseinfo:work.rightsreservedlicenseinfo:work.rightsreservedalle Rechte vorbehaltenall rights reserved/creativecommons/r/reserved/0.9/88x31.png[DE-28]Urheberrechtsschutz 1.0$gRights Statements$uhttp://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/http://rightsstatements.org/vocab/InC/1.0/licenseinfo:depositlicenseinfo:depositVeröffentlichungsgenehmigungpermission to storelicenseinfo:deposit.rightsgrantedlicenseinfo:deposit.rightsgrantedNutzungsrechte erteiltrights grantedlicenseinfo:metadatalicenseinfo:metadataLizenzen für Metadatenlicenseinfo:metadata.cc0licenseinfo:metadata.cc0Lizenz Metadaten: CC0license metadata: CC0/creativecommons/p/zero/1.0/88x31.pnghttps://creativecommons.org/publicdomain/zero/1.0/accesscondition:openaccessaccesscondition:openaccessfrei zugänglich (Open Access)open accesshttp://purl.org/coar/access_right/c_abf2OAfreeinfo:eu-repo/semantics/openAccess[DE-28]Open Access$gControlled Vocabulary for Access Rights$uhttp://purl.org/coar/access_right/c_abf2rfc5646:enrfc5646:enEnglischEnglishengengSimultaneous direct optimal controla versatile approach for steering quantum molecular dynamicsSimultaneous direct optimal controla versatile approach for steering quantum molecular dynamicsgnd:1365099962orcid:0009-0002-0922-1996gnd:141056487orcid:0000-0002-5132-2961gnd:1167532341orcid:0000-0001-8021-7063gnd:38329-6gnd:2147083-2gnd:1365099962orcid:0009-0002-0922-1996gnd:141056487orcid:0000-0002-5132-2961gnd:1167532341orcid:0000-0001-8021-7063gnd:38329-6gnd:2147083-2rosdok_disshab_0000003249-d2274012e53gnd:1365099962orcid:0009-0002-0922-1996Alejandro Rubenovich Ramos RamosAlejandro Rubenovich Ramos Ramosrosdok_disshab_0000003249-d2274012e69gnd:141056487orcid:0000-0002-5132-2961Oliver KühnOliver Kühnrosdok_disshab_0000003249-d2274012e86gnd:1167532341orcid:0000-0001-8021-7063Jean Christophe TremblayJean Christophe Tremblayrosdok_disshab_0000003249-d2274012e101gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000003249-d2274012e115gnd:2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätAlejandro Rubenovich Ramos RamosOliver KühnJean Christophe TremblayUniversität RostockUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätAlejandro Rubenovich Ramos RamosOliver KühnJean Christophe TremblayUniversität RostockUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätAlejandro Rubenovich Ramos RamosRostockUniversität Rostockepub.dissertationhttps://purl.uni-rostock.de/rosdok/id00004776urn:nbn:de:gbv:28-rosdok_id00004776-510.18453/rosdok_id00004776Controlling molecular processes by shaped laser pulses is a long-standing goal in Molecular Physics and Chemistry. Here, we suggest a direct optimal control approach based on a simultaneous simulation and optimization paradigm. This approach uses automatic differentiation, offering as advantages final time and model parameter optimization, as well as a wide range of terms in the performance functional and constraints that could be easily implemented in a plug-and-play fashion. The advantages of this approach will be showcased for diverse molecular model systems.20242024Enthält ZeitschriftenartikelOliver Kühn (University of Rostock) ; Jean Christophe Tremblay (University of Lorraine)[{"name":"Kühn, Oliver","affil":"University of Rostock"},{"name":"Tremblay, Jean Christophe","affil":"University of Lorraine"}]Dissertation, Universität Rostock, 2024, Kumulative Dissertationvorgelegt von Alejandro Rubenovich Ramos Ramosepub.dissertation1 Ramos_Ramos_Dissertation_2025.pdf 8637515 410081e8d96567b978f215ed83c27c1a rosdok/id000047761925256413Oau2025-05-092025-05-09T12:47:14ZrdaConverted from PICA to MODS using Pica2MODS XSLT Transformer 2.10 [SCM: "f6c168af690edb7cb65ef34e4a2bf7f8714c5d38" "v2.10" "2024-03-28T14:43:08+0100"] with mode 'DEFAULT'.DissertationHochschulschriftSimultaneous direct optimal controla versatile approach for steering quantum molecular dynamicsControlling molecular processes by shaped laser pulses is a long-standing goal in Molecular Physics and Chemistry. Here, we suggest a direct optimal control approach based on a simultaneous simulation and optimization paradigm. This approach uses automatic differentiation, offering as advantages final time and model parameter optimization, as well as a wide range of terms in the performance functional and constraints that could be easily implemented in a plug-and-play fashion. The advantages of this approach will be showcased for diverse molecular model systems.Alejandro RubenovichRamos Ramos1992 -VerfasserInaut13650999620009-0002-0922-1996OliverKühn1964 -AkademischeR BetreuerIndgs1410564870000-0002-5132-2961University of RostockJean ChristopheTremblayAkademischeR BetreuerIndgs11675323410000-0001-8021-7063University of Lorraine38329-6Universität Rostock1419 - 19761990 -Grad-verleihende Institutiondgg2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgghttps://purl.uni-rostock.de/rosdok/id00004776urn:nbn:de:gbv:28-rosdok_id00004776-510.18453/rosdok_id00004776530 Physik540 ChemieMathematisch-Naturwissenschaftliche Fakultätalle Rechte vorbehaltenNutzungsrechte erteiltLizenz Metadaten: CC0frei zugänglich (Open Access)en1 Online-Ressource (V, 89 Seiten)202418. März 2024Universität RostockRostockmonographic20242025Universitätsbibliothek RostockRostock2025Universitätsbibliothek Rostockhttps://purl.uni-rostock.de/rosdok/id00004776Enthält ZeitschriftenartikelOliver Kühn (University of Rostock) ; Jean Christophe Tremblay (University of Lorraine)[{"name":"Kühn, Oliver","affil":"University of Rostock"},{"name":"Tremblay, Jean Christophe","affil":"University of Lorraine"}]Dissertation, Universität Rostock, 2024, Kumulative Dissertationvorgelegt von Alejandro Rubenovich Ramos Ramos Kühn, Oliver University of Rostock Tremblay, Jean Christophe University of Lorraine 2025-05-09T12:29:47.631Z 2025-05-09T13:04:52.814Z 2025-05-19T13:04:52.862Z editorFG {"identifier":"rosdok/id00004776","type":"local_id","additional":"","service":"MCRLocalID","created":"2025-05-09T12:29:48.673Z"} {"identifier":"urn:nbn:de:gbv:28-rosdok_id00004776-5","type":"dnbUrn","additional":"","service":"RosDokURN","created":"2025-05-09T12:29:48.708Z"} {"identifier":"https://purl.uni-rostock.de/rosdok/id00004776","type":"purl","additional":"","service":"RosDokPURL","created":"2025-05-09T12:29:48.719Z","registrationStarted":"2025-05-09T13:04:51.311Z"} {"identifier":"10.18453/rosdok_id00004776","type":"doi","additional":"","service":"RosDokDOI","created":"2025-05-09T12:29:48.730Z","registrationStarted":"2025-05-09T13:04:50.800Z","registered":"2025-05-09T13:04:52.809Z"} MCRJANITORfulltextfile/rosdok_disshab_0000003249/rosdok_derivate_0000224328/Ramos_Ramos_Dissertation_2025.pdfSimultaneous direct optimal controla versatile approach for steering quantum molecular dynamicsSimultaneous direct optimal controla versatile approach for steering quantum molecular dynamicsgnd:1365099962orcid:0009-0002-0922-1996gnd:141056487orcid:0000-0002-5132-2961gnd:1167532341orcid:0000-0001-8021-7063gnd:38329-6gnd:2147083-2gnd:1365099962orcid:0009-0002-0922-1996gnd:141056487orcid:0000-0002-5132-2961gnd:1167532341orcid:0000-0001-8021-7063gnd:38329-6gnd:2147083-2rosdok_disshab_0000003249-d2274012e53gnd:1365099962orcid:0009-0002-0922-1996Alejandro Rubenovich Ramos RamosAlejandro Rubenovich Ramos Ramosrosdok_disshab_0000003249-d2274012e69gnd:141056487orcid:0000-0002-5132-2961Oliver KühnOliver Kühnrosdok_disshab_0000003249-d2274012e86gnd:1167532341orcid:0000-0001-8021-7063Jean Christophe TremblayJean Christophe Tremblayrosdok_disshab_0000003249-d2274012e101gnd:38329-6Universität RostockUniversität Rostockrosdok_disshab_0000003249-d2274012e115gnd:2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätAlejandro Rubenovich Ramos RamosOliver KühnJean Christophe TremblayUniversität RostockUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätAlejandro Rubenovich Ramos RamosOliver KühnJean Christophe TremblayUniversität RostockUniversität Rostock. Mathematisch-Naturwissenschaftliche FakultätAlejandro Rubenovich Ramos RamosRostockUniversität Rostockepub.dissertationhttps://purl.uni-rostock.de/rosdok/id00004776urn:nbn:de:gbv:28-rosdok_id00004776-510.18453/rosdok_id00004776Controlling molecular processes by shaped laser pulses is a long-standing goal in Molecular Physics and Chemistry. Here, we suggest a direct optimal control approach based on a simultaneous simulation and optimization paradigm. This approach uses automatic differentiation, offering as advantages final time and model parameter optimization, as well as a wide range of terms in the performance functional and constraints that could be easily implemented in a plug-and-play fashion. The advantages of this approach will be showcased for diverse molecular model systems.20242024Enthält ZeitschriftenartikelOliver Kühn (University of Rostock) ; Jean Christophe Tremblay (University of Lorraine)[{"name":"Kühn, Oliver","affil":"University of Rostock"},{"name":"Tremblay, Jean Christophe","affil":"University of Lorraine"}]Dissertation, Universität Rostock, 2024, Kumulative Dissertationvorgelegt von Alejandro Rubenovich Ramos Ramos[xslt]Saxonrosdok/id00004776https://purl.uni-rostock.de/rosdok/id00004776192525641310.18453/rosdok_id00004776urn:nbn:de:gbv:28-rosdok_id00004776-5Alejandro Rubenovich Ramos RamosRamos Ramos Alejandro RubenovichSimultaneous direct optimal control : a versatile approach for steering quantum molecular dynamicsDissertationdoctoral thesisUniversität Rostock, 18. März 2024Controlling molecular processes by shaped laser pulses is a long-standing goal in Molecular Physics and Chemistry. Here, we suggest a direct optimal control approach based on a simultaneous simulation and optimization paradigm. This approach uses automatic differentiation, offering as advantages…Alejandro Rubenovich Ramos RamosSimultaneous direct optimal controla versatile approach for steering quantum molecular dynamicsUniversitätsbibliothek Rostockhttps://purl.uni-rostock.de/rosdok/id00004776Alejandro RubenovichRamos Ramos1992 -VerfasserInaut13650999620009-0002-0922-1996OliverKühn1964 -AkademischeR BetreuerIndgs1410564870000-0002-5132-2961University of RostockJean ChristopheTremblayAkademischeR BetreuerIndgs11675323410000-0001-8021-7063University of Lorraine38329-6Universität Rostock1419 - 19761990 -Grad-verleihende Institutiondgg2147083-2Universität Rostock. Mathematisch-Naturwissenschaftliche FakultätGrad-verleihende Institutiondgg[purl]https://purl.uni-rostock.de/rosdok/id00004776[urn]urn:nbn:de:gbv:28-rosdok_id00004776-5[doi]10.18453/rosdok_id00004776open_access20242024epoch:21th_centuryrfc5646:endoctype:epub.dissertationaccesscondition:openaccessSDNB:530SDNB:540institution:unirostock.mnfstate:published