title: |
Laser control and spectroscopy of molecular vibrations and reaction dynamics |
|
contributing persons: |
Mateusz Lisaj[VerfasserIn] |
 |
1075019915 |
Oliver Kühn
, Prof. Dr.[AkademischeR BetreuerIn] |
 |
141056487 |
|
Universität Rostock, Institut für Physik |
Volkhard May
, PD Dr. habil.[AkademischeR BetreuerIn] |
 |
110000625 |
|
Humboldt-Universität zu Berlin, Institut für Physik |
|
contributing corporate bodies: |
Universität Rostock, Mathematisch-Naturwissenschaftliche Fakultät[Grad-verleihende Institution] |
 |
2147083-2 |
|
|
abstract: |
The main subjects of this work are the ultrafast laser driven quantum dynamics of
collective CO vibrations in a metal-dicarbonyl complex. The fundamental insights
into the interactions responsible for bond dissociation are obtained by using shaped
laser pulses to steer molecular quantum dynamics. Specifically, CpCo(CO)2 is studied
on the basis of a four-dimensional reactive potential energy surface (PES). It is
shown that two perpendicularly polarized IR laser pulses can be used to trigger an
alternating localization of the vibration within one CO bond.
[English] |
|
document type: |
|
institution: |
Faculty of Mathematics and Natural Sciences |
|
language: |
|
subject class (DDC): |
|
|
publication / production: |
Rostock: Universität Rostock
|
2015
|
|
|
identifiers: |
|
|
access condition: |
|
license/rights statement: |
all rights reserved This work may only be used under the terms of the German Copyright Law (Urheberrechtsgesetz). |
|
|
RosDok id: |
rosdok_disshab_0000001403 |
created / modified: |
05.08.2015 / 08.08.2023
|
metadata license: |
The metadata of this document was dedicated to the public domain (CC0 1.0 Universal Public Domain Dedication). |