Design, active sites and performance of unconventional ZrO2-based catalysts for non-oxidative dehydrogenation of C3 – C4 alkanes

Tatiana Otroshchenko

doi:10.18453/rosdok_id00002039

Tatiana Otroshchenko

Design, active sites and performance of unconventional ZrO2-based catalysts for non-oxidative dehydrogenation of C3 – C4 alkanes

Universität Rostock, 2018

https://doi.org/10.18453/rosdok_id00002039

Abstract: Catalytic non-oxidative dehydrogenation (DH) of C3 – C4 alkanes is of increasing importance due to the growing demand for the corresponding olefins. Commercial catalysts with supported CrOx or Pt-Sn species have, however, shortcomings of being toxic or limited availability. Against this background, the present thesis was focused on the development of alternative DH catalysts on the basis of metal oxides with usually unchangeable metal oxidation state but with high ability for lattice oxygen removal.

Dissertation Freier Zugang

Titel:

Design, active sites and performance of unconventional ZrO2-based catalysts for non-oxidative dehydrogenation of C3 – C4 alkanes

Beteiligte Personen:

Tatiana Otroshchenko[VerfasserIn]
	1154729516
Evgenii V. Kondratenko , PD Dr. habil.[AkademischeR BetreuerIn]
	1106565789
	Universität Rostock, Leibniz-Institut für Katalyse e.V.
Bert M. Weckhuysen , Dr. Ir.[AkademischeR BetreuerIn]
	Universität Utrecht, Inorganic Chemistry and Catalysis

Beteiligte Körperschaften:

Universität Rostock, Mathematisch-Naturwissenschaftliche Fakultät[Grad-verleihende Institution]
	2147083-2

Zusammenfassung:

Catalytic non-oxidative dehydrogenation (DH) of C3 – C4 alkanes is of increasing importance due to the growing demand for the corresponding olefins. Commercial catalysts with supported CrOx or Pt-Sn species have, however, shortcomings of being toxic or limited availability. Against this background, the present thesis was focused on the development of alternative DH catalysts on the basis of metal oxides with usually unchangeable metal oxidation state but with high ability for lattice oxygen removal. [Englisch]

Dokumenttyp:

Dissertation

Einrichtung:

Mathematisch-Naturwissenschaftliche Fakultät

Sprache:

Englisch

Sachgruppe der DNB:

540 Chemie

Veröffentlichung /
Entstehung:

Rostock

Rostock: Universität Rostock

2018